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If proto-Serbs and proto-Croats were Iranic tribes (there is very popular theory about that) than they probably were predominantly R1a-Z93.
I don't know from Croatians, but among Serbs there is 0% R1a-Z93.
In Serbia only few Hungarians from Vojvodina carry this haplogroup.
Maybe proto-Serbs and proto-Croats were some other branch of R1a.
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